Rheology of Carbon Fiber Thermoplastic Polymer Composites

By Byron Pipes

Purdue University

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The rheology of fiber–reinforced thermoplastic composites will be presented with specific focus on several topics studied over the past three decades. Interest in the elongational viscosity of collimated, discontinuous fiber systems was initiated by the introduction of impregnated, stretch broken fiber tow with the goal of establishing stretch forming forces. This work followed the classic solution by Bachelor in developing a micromechanics model for extensional viscosity of these systems for temperature dependent and shear thinning polymers. Next, the remaining individual components of the viscosity tensor, including the three shearing viscosities and the two additional elongational viscosities, were developed in a logical extension [1]. These models utilized the concept of hyper-concentrated systems and thereby provided rheological models for fiber concentrations significantly greater than conventional rheological models with dilute restrictions. This work was revised and extended to the flow of prepreg platelet systems consisting of planar reinforcing geometries and the absence of lubricating liquid matrices. The consolidation of the prepreg platelet systems, as the first stage of composite response to pressure gradients, was developed in order to establish the initial platelet geometry and fiber orientation state prior to molding flows [2]. Molding flows were then modeled for highly anisotropic viscosity tensors that changed with molding conditions such as mold geometry and flow path [3]. Validations of these simulations were demonstrated for both prepreg platelet systems and conventional sheet molding systems [4]. The more recent work focuses on the viscoelastic bending of collimated fiber systems with application to both continuous and discontinuous fiber systems. The target applications are flexural deformation in sheet forming and extrudate rheology in extrusion deposition additive manufacturing. Finally, an attempt to anticipate what advances will be developed in the next three decades will be described.

1. Pipes, R. B., Coffin, D. W., Simacek, P., Shuler, S. F., and Okine, R. K., “Rheological Behavior of Collimated Fiber Thermoplastic Composite Materials,” Flow Phenomena in Polymeric Composites, edited by S. G. Advani, R. B. Pipes, Series Editor, Elsevier Science Publishers, (1994), pp. 85-125. 2. Sommer, Drew E., Sergii G. Kravchenko, and R. Byron Pipes. “A numerical study of the meso-structure variability in the compaction process of prepreg platelet molded composites.” Composites Part A: Applied Science and Manufacturing 138 (2020): 106010. 3. Favaloro, A.J., Tseng, H-C., Pipes, R.B., A new anisotropic viscous constitutive model for composites molding simulation, Composites Part A, 115, (2018), pp. 112–122. 4. Favaloro, A.J., Sommer, D.E., Denos, B.R. and Pipes, R.B., “Simulation of Prepreg Platelet Compression Molding: Method and Orientation Validation,” J. Rheo., Vol. 62, No. 6 (2018), pp. 1443-1455.

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Researchers should cite this work as follows:

  • Byron Pipes (2021), "Rheology of Carbon Fiber Thermoplastic Polymer Composites," https://cdmhub.org/resources/1968.

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Wenbin Yu

Purdue University